Publications

This article demonstrates that 3D-printed parts can replace metal parts in optomechanics in the correct circumstances. Three examples are shown: a clamping fork for pedestal holders where stability is important, an adjustable mirror holder where the rigidity is the main criterion, and a stray light shield where the transmissivity is critical. By combining carbon-fiber-reinforced polymers (CFRPs) with 3D printing, it is possible to produce components that fill the gap between standard 3D-printed plastics and metal parts in terms of strength and stability. These parts are designed to be lighter, more compact, and easier to modify, while keeping good mechanical properties such as resistance to vibration, shape accuracy, and controlled thermal expansion. The article focuses on the application of composite 3D printing on optomechanical components. It compares different methods of composite 3D printing, including fused filament fabrication (FFF) with either chopped fibers or with continuous fiber reinforcement. Three examples from the HiLASE Centre demonstrate how these parts are used in practice, confirming that it is indeed possible to 3D print components that are lighter and cheaper yet still highly functional compared to their off-the-shelf counterparts—for example, lightweight and stiff mounts, shielding against stray laser light, or flexible elements allowing fine mechanical adjustments. Simulations of the deformations are included to compare the printed and metal versions. The article ends with a summary of the benefits and limitations of using 3D-printed composites in optomechanics.

We present an active alignment and stabilization control system for laser setups based on a thin-disk regenerative amplifier. This method eliminates power and pointing instability during the warm-up period and improves long-term stability throughout the entire operation. The alignment method is based on a four-mirror control system consisting of two motorized mirrors placed within the regenerative amplifier cavity, two additional motorized mirrors external to the amplifier cavity, and four camera detectors. The implemented stabilization system achieves significant performance improvements, increasing the power stability from 1.87% to 0.79% RMS and the peak-to-peak stability from 7.43% to 3.88%. Furthermore, the system significantly enhances beam positional stability, achieving up to a sixfold improvement in certain sensor measurements. The advantage of this method is the removal of long-term pointing instability by adding a second controlled motorized mirror to the cavity, in addition to using only one cavity end mirror for optimizing the overlap with the pump spot on the cavity medium. To achieve higher precision in pointing, the nonlinear hysteresis effect of the piezoelectric actuator is mitigated. Although the power and pointing stability of the cavity are secured, pointing instability at the input of the compressor occurs. This issue is resolved by two additional controlled motorized mirrors external to the cavity.

Controlling microbial adhesion in industrial and healthcare settings is crucial for maintaining hygiene and preventing biofilm formation. This work describes a novel method to efficiently produce yeast adhesion-reducing surfaces using dynamic beam-shaping with a spatial light modulator. At first, the laser-induced periodic surface structures (LIPSS) topography was tuned to test microbial adherence in a variety of LIPSS configurations, specifically using Saccharomyces cerevisiae as a model organism. A novel and robust dual-pass laser strategy was implemented to create hierarchical LIPSS structures with periodicities of 630 nm and 5 μm. The integration of dynamic beam shaping with spatial light modulator (SLM) significantly enhanced production efficiency, achieving a throughput of up to 150 cm2/min. The laser-structured surfaces exhibited a significant reduction in yeast adhesion, with a decrease of 95% in adherent cells and achieving a maximum reduction of 99.88%. These findings offer promising implications for developing advanced surface treatments to improve hygiene in industries such as food processing and healthcare, where minimizing microbial colonization is vital.

Micro-geometrical errors, surface roughness, and surface integrity (microstructure, residual stresses, microhardness) play an important role in defining the quality of the gears as they directly affect their noise, vibration characteristics and service life during their use. In the present work, underwater laser shock peening (LSP) is employed to improve the quality of the laser powder bed fusion built 17-4 PH small-size spur gears (12 mm outside diameter). LSP was employed near the spur gear root, and effects were measured in terms of residual stresses, variation in microgeometry errors, surface roughness, porosity, microstructure, and microhardness. It was observed that LSP could impart compressive residual stresses up to 0.4 mm of measured depth, while the surface roughness has improved by 32%. Microgeometry and microhardness of gears showed minor variations. Additionally, LSP has shown an impact on the microstructure as the grain orientation was altered and grain size reduced by 15.6% due to shock wave transmission. The study paves the way to use LSP as a post-processing technique to modify the surface characteristics of LPBF-built miniature spur gears with minimal impact on the gear microgeometry.

In this work Laser Peening without Coating (LPwC) was applied underwater on heterogeneous weld joint made of P265GH and X6CrNiTi18-10 steel tubes to prevent Environmental Assisted Cracking on the weld/P265GH steel fusion boundary. Special laser head was designed to precisely deliver 200 mJ green laser beam on the centrally located weld interface on the inner surface of a pipe 76 mm wide and 420 mm long. Residual stress analysis revealed that the LPwC treatment led to generation of compressive residual stresses in the critical fusion boundary area with the magnitude of −168 MPa despite the absence of a protective layer in the peening process. The depth of compressive stresses reached up to 0.8 mm. Plastic deformation induced by LPwC led to grain refinement in the microstructure and improved hardness by 16 %. Samples sectioned from the treated pipe were subjected to accelerated corrosion-mechanical testing which showed more than 2.5x increase in cycles to failure after LPwC. Fractography analysis showed shorter length and decreased number of corrosion cracks after LPwC as well as formation of protective oxide layer on top of the treated surface. 3-point bend testing further showed more than 8x increase in corrosion fatigue life.

The process of silver cluster formation in a rarefied supersonic jet of a mixture of silver vapor with helium carrier gas is investigated. The study was carried out by the direct simulation Monte Carlo method and a kinetic model of cluster growth. Two simplified geometries of the jet source are considered. The data on cluster size distributions and gasdynamic parameters of the mixture species (metal and carrier gas atoms, metal clusters) are presented for a wide range of the mole fraction of helium in the source. The impact of kinetic model parameters on the flow pattern and cluster formation process are analyzed. The modeling results are compared with available experimental data.

An experimental and theoretical study of laser-induced damage and ablation of silicon by two individual femtosecond pulses of different wavelengths, 1030 and 515 nm, is performed to address the physical mechanisms of dual-wavelength ablation and reveal possibilities for increasing the ablation efficiency. The produced craters and damaged areas are analyzed as a function of laser fluence and time separation between the pulses and are compared with monochromatic irradiation. The order of pulses is demonstrated to be essential in bi-color ablation with higher material removal rates when a shorter-wavelength pulse arrives first at the surface. Simulations based on the two-temperature model show that the visible pulse is profitable for the generation of the electron-hole plasma while the delayed IR pulse is efficiently absorbed in the plasma enhancing energy coupling to the target. At long delays of 30–100 ps, the dual-wavelength ablation is found to be particularly strong with formation of deep smooth craters. This is explained by the expansion of a hot liquid layer produced by the first pulse with a drastic decrease in the surface reflectivity at this timescale. The results provide insight into the processes of dual-wavelength laser ablation offering a better control of the energy deposition into material.

High entropy alloys (HEAs) have a wide range of applications across various fields, including structural engineering, biomedical science, catalysis, magnetism, and nuclear technology. Nanoscale HEA particles show promising catalytic properties. Nevertheless, attaining versatile composition control in nanoparticles poses a persistent challenge. This study proposes the use of pulsed laser ablation in liquids (PLAL) for synthesizing nanoparticles using equiatomic CoCrFeMnNi targets with varied preparation methods. We evaluate the impact of target preparation method on nanoparticle yield and composition as well as the magnetic properties of the nanoparticles. The elemental powder-pressed heat-treated target (HEA-PP), identified as the most time-efficient and cost-effective, exhibits noticeable segregation and non-uniform elemental distribution compared to ball milled hot-pressed powder (HEA-BP) and face-centered cubic (FCC) single crystal (HEA-SX) alloy targets. From all targets, nanoparticles (sizes from 2 to 120 nm) can be produced in ethanol with a nearly equiatomic CoCrFeMnNi composition and a FCC structure, showing oxidation of up to 20 at.%. Nanoparticles from HEA-PP exist in a solid solution state, while those from HEA-BP and HEA-SX form core-shell structures with a Mn shell due to inhomogeneous material expulsion, confirmed by mass spectrometry. HEA-PP PLAL synthesis demonstrates 6.8 % and 15.1 % higher productivity compared to HEA-BP and HEA-SX, establishing PLAL of elemental powder-pressed targets as a reliable, time-efficient, and cost-effective method for generating solid solution HEA nanoparticles.

Volumetric modification of dielectrics by ultrashort laser pulses is a complex dynamic phenomenon involving material photoexcitation and associated nonlinear processes. To achieve control over modification, it is necessary to gain a deep insight into the dynamics of laser-excited processes that can be realized using double-laser-pulse experiments with different time separations supported by numerical simulations. In this paper, we apply this approach to investigate fused silica modification with femtosecond laser pulses that provides time-resolved information about the dynamic behavior of the laser-excited bandgap material. It is shown that the laser-generated free-electron plasma causes a shielding effect for the following pulse with a characteristic duration of ∼600 fs after the pulse action. Within this time interval, the second pulse produces a reduced modification as compared to a longer time separation between pulses. For double pulses with different energies, it was found that the volumetric modification is stronger when a lower-energy pulse couples with material first. This is explained by the combination of the effects of the re-excitation of self-trapped excitons, which are generated as a result of free electron recombination and associated light shielding. Experimental results are supported by numerical simulations of double laser pulse propagation in nonlinear media based on Maxwell’s equations. Our findings offer a route for better controlling the inscription of 3D photonic structures in bulk optical materials.

Pulsed laser ablation in liquids (PLAL) is a versatile technique to produce high-purity colloidal nanoparticles. Despite considerable recent progress in increasing the productivity of the technique, there is still significant demand for a practical, cost-effective method for upscaling PLAL synthesis. Here we employ and unveil the fundamentals of multi-beam (MB) PLAL. The MB-PLAL upscaling approach can bypass the cavitation bubble, the main limiting factor of PLAL efficiency, by splitting the laser beam into several beams using static diffractive optical elements (DOEs). A multimetallic high-entropy alloy CrFeCoNiMn was used as a model material and the productivity of its nanoparticles in the MB-PLAL setup was investigated and compared with that in the standard single-beam PLAL. We demonstrate that the proposed multi-beam method helps to bypass the cavitation bubble both temporally (lower pulse repetition rates can be used while keeping the optimum processing fluence) and spatially (lower beam scanning speeds are needed) and thus dramatically increases the nanoparticle yield. Time-resolved imaging of the cavitation bubble was performed to correlate the observed production efficiencies with the bubble bypassing. The results suggest that nanoparticle PLAL productivity at the level of g/h can be achieved by the proposed multi-beam strategy using compact kW-class lasers and simple inexpensive scanning systems.

Ultrafast laser processing possesses unique outlooks for the synthesis of novel nanoarchitectures and their further applications in the field of life science. It allows not only the formation of multi-element nanostructures with tuneable performance but also provides various non-invasive laser-stimulated modalities. In this work, we employed ultrafast laser processing for the manufacturing of silicon–gold nanocomposites (Si/Au NCs) with the Au mass fraction variable from 15% (0.5 min ablation time) to 79% (10 min) which increased their plasmonic efficiency by six times and narrowed the bandgap from 1.55 eV to 1.23 eV. These nanostructures demonstrated a considerable fs laser-stimulated hyperthermia with a Au-dependent heating efficiency (~10–20 °C). The prepared surfactant-free colloidal solutions showed good chemical stability with a decrease (i) of zeta (ξ) potential (from −46 mV to −30 mV) and (ii) of the hydrodynamic size of the nanoparticles (from 104 nm to 52 nm) due to the increase in the laser ablation time from 0.5 min to 10 min. The electrical conductivity of NCs revealed a minimum value (~1.53 µS/cm) at 2 min ablation time while their increasing concentration was saturated (~10¹² NPs/mL) at 7 min ablation duration. The formed NCs demonstrated a polycrystalline Au nature regardless of the laser ablation time accompanied with the coexistence of oxidized Au and oxidized Si as well as gold silicide phases at a shorter laser ablation time (<1 min) and the formation of a pristine Au at a longer irradiation. Our findings demonstrate the merged employment of ultrafast laser processing for the design of multi-element NCs with tuneable properties reveal efficient composition-sensitive photo-thermal therapy modality.

Traditionally, single-color laser beams are used for material processing and modifications of optical, mechanical, conductive, and thermal properties of different materials. So far, there are a limited number of studies about the dual-wavelength laser irradiation of materials, which, however, indicate a strong enhancement in laser energy coupling to solid targets. Here, a theoretical study is reported that aimed at exploring the volumetric excitation of fused silica with dual-wavelength (800 nm and 400 nm) ultrashort laser pulses focused on the material’s bulk. Numerical simulations are based on Maxwell’s equations, accounting for the generation of conduction electrons, their hydrodynamic motion in the laser field, and trapping into an excitonic state. It is shown that, by properly choosing the energies of the two laser harmonics successively coupling with the material, it is possible to strongly enhance the laser energy absorption as compared to the pulses of a single wavelength with the same total energy. Laser energy absorption strongly depends on the sequence of applied wavelengths, so that the shorter wavelength pre-irradiation can yield a dramatic effect on laser excitation by the following longer-wavelength pulse. The predictions of this study can open a new route for enhancing and controlling the highly localized absorption of laser energy inside transparent materials for optoelectronic and photonic applications.

The objective of this work is to study the effects of different coating materials (black paint, thermoplastic elastomers, black vinyl tape and uncoated surfaces) in Laser Shock Peening (LSP) processing of laser powder bed fusion (L-PBF) printed thin AlSi10Mg tubes. The investigations were carried out with pre-identified optimal LSP parameters for the AlSi10Mg material. The study was performed using an analysis of surface residual stresses, where a maximum compressive stress of −85 MPa has been reached, while the depth of the compressive regime stays till 2 mm. The microstructural study reveals the multifold dislocation of the grains and formation of new sub-grains, thus changing the grain boundaries in all experiments due to lattice strain development by LSP. Microhardness has also shown alteration after LSP and accounted for a 5–15% increase in it after LSP. Surface properties, such as roughness and volumetric parameters, have also shown changes after LSP processing.

In this paper, we present a single crystal, KTA (potassium titanyl-arsenate, KTiOAsO₄) based picosecond optical parametric amplifier pumped by an in-house built 1030 nm Yb:YAG thin-disk laser, capable of tunability from 1.46 to 3.5 µm, operating at 90 kHz, with high average power in the signal and idler beams. The highest output power of 8.9 W was reached for the 1750 nm signal beam with 19% conversion efficiency and the respective 2500 nm idler beam power was 6.2 W with 13% efficiency. The highest combined signal and idler mid-infrared power was 17 W at the 2060 nm wavelength degeneracy point.

We report on stable, long-term operation of a diode-pumped solid-state laser (DPSSL) amplifying 15 ns pulses at 1029.5 nm wavelength to 10 J energy at 100 Hz pulse rate, corresponding to 1 kW average power, with 25.4% optical-to-optical efficiency. The laser was operated at this level for over 45 minutes (∼3 · 10⁵/ shots) in two separate runs with a rms energy stability of 1%. The laser was also operated at 7 J, 100 Hz for 4 hours (1.44 · 10⁶/ shots) with a rms long-term energy stability of 1% and no need for user intervention. To the best of our knowledge, this is the first time that long-term reliable amplification of a kW-class high energy nanosecond pulsed DPSSL at 100 Hz has been demonstrated.

<em>We studied the effect of Ga³⁺and Sc³⁺ on Yb:YAG emission at cryogenic temperatures on three different mixed garnets namely Yb:YGAG, Yb:YSAG and Yb:YSGAG. The compositional tuning of these mixed garnets was achieved by preparing ceramic pellets by solid state reaction with different concentration of Ga³⁺, or Sc³⁺, or both. The incorporation of Sc³⁺ in Yb:YAG leads only to a limited spectral broadening. On the other hand, the incorporation of either Ga³⁺ or both Ga³⁺ and Sc³⁺ results in a significant spectral broadening. In the latter case, this inhomogeneous broadening is attributed to the mixed occupancy of both Ga³⁺ and Sc³⁺ in octahedral and tetragonal sites in the crystal lattice leading to a significant distortion in the structure.</em>

An experimental platform for laser-driven ion (sub-MeV) acceleration and potential applications was commissioned at the HiLASE laser facility. The auxiliary beam of the Bivoj laser system operating at a GW level peak power (~10 J in 5–10 ns) and 1–10 Hz repetition rate enabled a stable production of high-current ion beams of multiple species (Al, Ti, Fe, Si, Cu, and Sn). The produced laser–plasma ion sources were fully characterized against the laser intensity on the target (1013–1015 W/cm2) by varying the laser energy, focal spot size, and pulse duration. The versatility and tuneability of such high-repetition-rate laser–plasma ion sources are of potential interest for user applications. Such a statistically accurate study was facilitated by the large amount of data acquired at the high repetition rate (1–10 Hz) provided by the Bivoj laser system.

The industry's demand for intricate geometries has spurred research into additive manufacturing (AM). Customising material properties, including surface roughness, integrity and porosity reduction, are the key industrial goals. This necessitates a holistic approach integrating AM, laser shock peening (LSP) and non-planar geometry considerations. In this study, machine learning and neural networks offer a novel way to create intricate, abstract models capable of discerning complex process relationships. Our focus is on leveraging the certain range of laser parameters (energy, spot area, overlap) to identify optimal residual stress, average surface roughness, and porosity values. Confirmatory experiments demonstrate close agreement, with an 8% discrepancy between modelled and actual residual stress values. This approach's viability is evident even with limited datasets, provided proper precautions are taken.

This article deals with the effect of strain-assisted tempering (SAT) on the fatigue properties of 54SiCr6 steel used for spring steel wires in a wide variety of automotive applications, including coil springs. This steel spring wire is extremely strong, having a high elastic limit and yield point, giving the steel excellent energy accumulation and fatigue properties. This combination opens up new possibilities in helical and cylindrical coil spring design, resulting in the reduction of both size and weight. Lightweight coil springs lead to improvements in fuel consumption, stability and vehicle traction. A large plastic deformation and SAT were applied to enhance the yield point of the study material. Improvements in the static and cyclic properties of steel springs were investigated using tensile tests and 3PB fatigue tests at ambient temperature. In addition, an advanced laser shock peening (LSP) process was employed to increase the fatigue resistance of the SAT material. The results presented here show great improvements in the static and fatigue properties over commercial steel treatment. The material quality of the wires was evaluated to be insufficient for further processing with cold coiling.

A systematic experimental study was performed to determine laser irradiation conditions for the large-area fabrication of highly regular laser-induced periodic surface structures (HR-LIPSS) on a 220 nm thick Mo film deposited on fused silica. The LIPSS were fabricated by scanning a linearly polarized, spatially Gaussian laser beam at 1030 nm wavelength and 1.4 ps pulse duration over the sample surface at 1 kHz repetition rate. Scanning electron microscope images of the produced structures were analyzed using the criterion of the dispersion of the LIPSS orientation angle (DLOA). Favorable conditions, in terms of laser fluence and beam scanning overlaps, were identified for achieving DLOA values <10°. To gain insight into the material behavior under these irradiation conditions, a theoretical analysis of the film heating was performed, and surface plasmon polariton excitation is discussed. A possible effect of the film dewetting from the dielectric substrate is deliberated.